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A universal synthesis strategy for P-rich noble metal diphosphide-based electrocatalysts for the hydrogen evolution reaction

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成果类型:
期刊论文
作者:
Pu, Zonghua;Zhao, Jiahuan;Amiinu, Ibrahim Saana;Li, Wenqiang;Wang, Min;...
通讯作者:
Mu, Shichun
作者机构:
[Mu, Shichun; Li, Wenqiang; Amiinu, Ibrahim Saana; Pu, Zonghua; He, Daping; Zhao, Jiahuan; Wang, Min] Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, Wuhan 430070, Hubei, Peoples R China.
[He, Daping] Wuhan Univ Technol, Hubei Engn Res Ctr RF Microwave Technol & Applica, Wuhan 430070, Hubei, Peoples R China.
通讯机构:
[Mu, Shichun] W
Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, Wuhan 430070, Hubei, Peoples R China.
语种:
英文
期刊:
Energy & Environmental Science
ISSN:
1754-5692
年:
2019
卷:
12
期:
3
页码:
952-957
基金类别:
This work was supported by the National Natural Science Foundation of China (51672204). We express heartfelt thanks to Prof. Gaoke Zhang for the supply of computational resources in the School of Resources and Environmental Engineering, Wuhan University of Technology. The authors also wish to sincerely thank the anonymous reviewers for their constructive review remarks and valuable suggestions.
机构署名:
本校为第一且通讯机构
院系归属:
材料复合新技术国家重点实验室
湖北省射频微波应用工程技术研究中心
摘要:
Highly efficient, stable and cost-efficient electrocatalysts for hydrogen generation via water splitting have become in increasing demand for future energy systems. Hitherto, P-rich noble metal polyphosphides which can decrease noble metal (such as Rh, Pd, or Ir) dosage are important to probe potential high-performance HER electrocatalysts. Nevertheless, they are difficult to synthesize at ambient pressure and moderate temperatures. Herein, for the first time, we report a novel iridium diphosphide (IrP2) electrocatalyst embedded within an ultra...

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