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Novel photoactivation promoted light-driven CO2 reduction by CH4 on Ni/CeO2 nanocomposite with high light-to-fuel efficiency and enhanced stability

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成果类型:
期刊论文
作者:
Zhang, Qian;Mao, Mingyang;Li, Yuanzhi*;Yang, Yi;Huang, Hui;...
通讯作者:
Li, Yuanzhi
作者机构:
[Wu, Shaowen; Jiang, Zhongkai; Mao, Mingyang; Huang, Hui; Zhao, Xiujian; Li, Yuanzhi; Zhang, Qian; Hu, Qianqian; Yang, Yi] Wuhan Univ Technol, State Key Lab Silicate Mat Architectures, 122 Luoshi Rd, Wuhan 430070, Hubei, Peoples R China.
通讯机构:
[Li, Yuanzhi] W
Wuhan Univ Technol, State Key Lab Silicate Mat Architectures, 122 Luoshi Rd, Wuhan 430070, Hubei, Peoples R China.
语种:
英文
关键词:
CO2 reduction by CH4;Light-to-fuel efficiency;Ni/CeO2 nanocomposite;Photocatalytic;Photothermocatalytic
期刊:
Applied Catalysis B: Environmental
ISSN:
0926-3373
年:
2018
卷:
239
页码:
555-564
基金类别:
This work was supported by National Natural Science Foundation of China ( 21673168 , 21473127 ). Q. Zhang and Dr. M. Y. Mao have same contribution to the paper.
机构署名:
本校为第一且通讯机构
院系归属:
硅酸盐建筑材料国家重点实验室
摘要:
The catalytic CO2 reduction by CH4 to synthesize fuels of CO and H2 (CRM) supplies a prospective technology to address the global warming effect caused by greenhouse gas of CO2. Due to its highly endothermic characteristics, CRM can only proceed at high reaction temperature, resulting in excessive energy consumption and quick catalyst deactivation due to serious carbon. Herein, we report a nanocomposite of Ni/CeO2 that exhibits high catalytic activity and good stability with focalized UV–vis-Infrared (UV–vis-IR) illumination without applying ...

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